Passivation of the Buried Interface via Preferential Crystallization of 2D Perovskite on Metal Oxide Transport Layers

Published in Advanced Materials 2021, 33 (41), e2103394, 2021

Organic spacer cations bearing −NH2 groups preferentially bind to under-coordinated oxygens on metal oxide substrates, inducing spontaneous 2D perovskite crystallization at the buried interface that reduces surface recombination velocity by 72% and enables up to 22.9% PCE in inverted solar cells.

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Recommended citation: Chen, B.; Chen, H.; Hou, Y.; Xu, J.; Teale, S.; Bertens, K.; Chen, H.; Proppe, A.; Zhou, Q.; Yu, D.; Xu, K.; Vafaie, M.; Liu, Y.; Dong, Y.; Jung, E. H.; Zheng, C.; Zhu, T.; Ning, Z.; Sargent, E. H. Passivation of the Buried Interface via Preferential Crystallization of 2D Perovskite on Metal Oxide Transport Layers. Advanced Materials 2021, 33 (41), e2103394.
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